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Darvond: Hold on, let me just pick one song from the 10,000+ from my collection.
good luck with that :P
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tinyE: Oh I forgot, Carmageddon 2.
Caramgeddon 1 sound like someone farting in a bottle!
Pick one...? Are you crazy? Here's a few in no particular order. Not necessarily my top faves, but easy ones.

NieR Automata: Birth of a Wish (Become as Gods/This Cannot Continue)

The Elder Scrolls V: Skyrim: Dovahkiin (For that matter, Morrowind and Oblivion too)

Final Fantasy VII: One Winged Angel
Good soundtracks, most games by Jesper Kyd like the Hitman games he worked on.
Mace Griffin Bounty Hunter, Blade of Darkness, Outcast, Interstate 76.

https://www.youtube.com/watch?v=3ttdJtEcSmA

https://www.youtube.com/watch?v=l3si8jkva_U

https://www.youtube.com/watch?v=GbBB_w-ivdc&list=PLZsxw2L9A0od00tt0M8GCGXE60Zwx0Gif&index=45

https://www.youtube.com/watch?v=tkhv-sMTeI0

https://www.youtube.com/watch?v=FiqeX59afAw

https://www.youtube.com/watch?v=WjW0KYVZFFk
One of the soundtracks that stands out for me the most.

Sonic the Hedgehog 2 Full Soundtrack
https://www.youtube.com/watch?v=YKuPQzhk8rY

Me and a friend of mine spent several weekends drunk, high and out of our minds playing it on his Genesis. When we couldn't get a ride to a party, or sneak out to go somewhere else, this game (along with Rampart and Outlander) burned through our free time. The music still takes me back instantly to the early/mid 90s.
ROLLING STAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAAA

https://www.youtube.com/watch?v=pls6OyJpCWg
Surprised no one mentioned Command & Conquer yet.

Command -&- Conquer OST - 15 - Mechanical Man (Target)
Too many. I tend to have a video game playlist branching from all eras of gaming. Dune 2000 has a good soundtrack though.
Best song:

Two Worlds - Play the Game
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Hyperborean111: Best song:

Two Worlds - Play the Game
Oh yes. Can say it's the first time I really just spent time on the menu of a game specifically to listen to the song, and tended to wait at least for a chorus whenever I started it up, before loading my last save to continue. The fact that it has vocals is quite a requirement for that, and darn few games have that, especially where you can just sit and listen, not only possibly at the end.

Edit: Pardon, had timeline mixed up, first was Baba Yetu. But while the initial reaction was similar, don't remember actually waiting to listen to it every time I started up the game quite so much though. And played Civ4 for a whole lot less time than TW, first the computer really struggled with it but still wanted to just win once, then when I built a better computer gave it another go, won one more time, and that was it. In TW the in-game timer said over 100h at the end, took me quite a while.
Post edited April 16, 2019 by Cavalary
These are the game tracks I listen to most often:


Rogue Trooper (specifically, Track 1)
Game page: https://www.gog.com/game/rogue_trooper
(some of the audio from that track is in the gameplay video on the game page)

Rogue Trooper Redux version (the collector's edition also has the soundtrack):
Game Page https://www.gog.com/game/rogue_trooper_redux_collectors_edition


Trine (the whole soundtrack)
Game Page https://www.gog.com/game/trine_enchanted_edition


Cosmo's Cosmic Adventure (specifically the Da Do Da - special stage track)
Game Page https://www.gog.com/game/cosmos_cosmic_adventure
that song on youtube: https://youtu.be/bNVucD9y9-4


Katamari Damacy soundtrack

Halo soundtrack
Grim Fandango and Gabriel Knight 3 have a great OST too.
Donkey Kong 64 has some very nice boss music.

Star Ocean 2 has Rena's theme in its variations. (This is one of the reasons I prefer to play as Rena in that game, though you do get to hear this theme as Claude.)

Secret of Mana has some nice music; my favorite is Still of the Night (plays in that beautiful forest area you visit near the end of the game, and which you unfortunately can't revisit after clearing).

Zelda has some nice music. Stone Tower Temple from Majora's Mask, the ruins theme from Oracle of Seasons, and for more recent examples, the final dungeon themes for both Link Between Worlds and Breath of the Wild.

Getting a bit more modern, there's Heaven's Prayer from Dragon Quest 9. That series has some other good music, including DQ1's world map theme, and the normal battle themes for DQ3, DQ4 (both of them!), and DQ5.

Of course, the Final Fantasy series also has nice music. Final Fantasy 2 has a really beautiful (though sad) overworld theme, and FF3 also has the music for the flooded world (which unfortunately you don't get to hear much). FF3 also has the Nepto Shrine theme as well as Covert Village Falgabard (which also plays in a couple other optional towns). FF3 also has that theme that plays in both that tree dungeon and the cave of darkness. FF5 has its final overworld theme, as well. There's more great FF music, but I think I'll stop here.

For more recent indie games:

Hollow Knight's entire soundtrack is really good (probably my favorite modern indie game soundtrack).

Tangledeep has one track I like, Child of the Forest (Shara's Theme), which is really beautiful. (It plays in the safe area after the second boss, and in the DLC it's used for the first area (Cedar Caverns) in Shara's story.
Hollow Knight's Soundtrack is by far the most memorable for me. Sealed Vessel is such a phenomenal track. Christopher Larkin really kills it. I can't wait to see what he has in store for Silksong.
Way too many to list...

If I had to pick one, it would probably be "When Gods Fall" from Titan Quest soundtrack.