TL;DR: Mod crashes on the opening cutscene. After the deletion of every single file related to Fallout 4, multiple fresh installs, flat-out uninstalling other modding programs, and attempted suggested fixes/mods for stability, and doing my damndest to get this running, it simply will not go past the first cutscene. Immediately crashes, doesn't respond to Alt+F4, displays over Task Manager, and this is the worst modding experience I've had in my 20 years of doing it. So much for "easy install" mods on GoG.