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My standard recommendation for kids, Viva Pinata.

And you can't really go wrong with the Sims.
If you get a 3DS, Pokemon would be a must.
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Roxolani: Also, are Wii U and Nintendo 3DS suitable for little kids?
I'd be careful with the 3DS, depending on the age of the children; Nintendo themselves avise against using the 3D feature if they are under 6 years old.
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bad_fur_day1: My standard recommendation for kids, Viva Pinata.

And you can't really go wrong with the Sims.
I wouldn't exactly go and suggest a game that's gotten a T rating since it first hit shelves. (Nor would I want to support EA.)